Wouldn't something like eSATA be a better choice? The hdd's speed would be the limiting factor instead of the bus.
So, for the kind of use case where you need to move lots of data, very quickly, eSATA may not be better :)
Edit: The g-raid mentioned looks like a 2x spinning array, so well within the limits of a single sata III bus.
Also, aside from the G-Raid, we also use 1 and 2tb SSD's (more for portability than the extra speed).