My son liked Fishtronaut / Peixonauta [1] which was made in Brazil and released in Portuguese, Spanish, and English simultaneously, I think (it's on Netflix in the US).

1: http://tvpinguim.com/peixonauta/

Obrigado! We found a few kids shows - Palavra Cantada has a great channel on there, and there are a few Turma da Monica episodes.

But not films like Toy Story.