There have been solutions to this problem with urban farming practices with a combination of hydroponics and vermiponics for a number of years which can grow quite a bit of usable produce in a smaller land area using significantly less water.
Also, it could be useful to continue to break down these statistics by crop and water use. For instance, almond farms appear to take up nearly 10% of California's water use (http://www.slate.com/articles/technology/future_tense/2014/0...).
Doing so would lend credence to which crop would be most effective for first improving upon. This report appears to suggest that alfalfa is one of the neediest crops grown in California in terms of water consumption. There are obvious other crops as well, in terms of land area (Corn being one of them) but nevertheless it's worth noting. https://www.arb.ca.gov/fuels/lcfs/workgroups/lcfssustain/han...
Now, you might be asking, what is alfalfa for? Alfalfa is grown as a feed for animals, mainly dairy cows. Dairy cows eat roughly 70% of the alfalfa produced in the US. It's important to note that some alfalfa farmers tend to disagree that solutions like drip irrigation will work effectively enough - as it sometimes depends on the soil type and exposure to critters chewing up the pipes. (http://www.kpbs.org/news/2015/jul/03/how-one-california-alfa...)