I'm not sure I understand how switching someone from Windows+Office to Ubuntu+LibreOffice is a security win. LibreOffice is not an especially safe piece of software.
* It doesn't have all that macro bundling stuff in normal documents that's the source of the whole macrovirus issue.
* It doesn't have any OLE-object-can-run-embedded-EXE-files-on-click-feature.
I'd say that's a huge win.
VServer or similar could also work well but might be harder to configure correctly.
Also modern versions of Office already run in a sandbox on Windows (AppContainer?) so how much are you really gaining?