I think it really depends on personal preference. I have stayed away from using the larger CSS frameworks. I won't mention them because I don't think it's right to "call out" CSS frameworks when its just my own personal usage of some frameworks over others.
I will mention ones that I have used:
Bootstrap ( http://getbootstrap.com/ )
Semantic UI ( https://semantic-ui.com/ )
Skeleton ( http://getskeleton.com/ )
GetFlakes ( http://getflakes.com )
Milligram ( http://milligram.github.io/ )
HackCSS ( http://hackcss.com/ )
Furtive ( http://furtive.co/ )
BassCSS ( http://basscss.com/ )
w3.css ( https://www.w3schools.com/w3css/ )
Spectre ( https://picturepan2.github.io/spectre/ )
CaiuSS ( http://ionicabizau.github.io/CaiuSS/ )
I really like the stuff and fluff Spectre offers: cards, navigation bar, etc.
Pure's grid is what I use exclusively. Simple, easy, and targets the screen sizes I want,