Have you performance benchmarked this? Would be interested in giving it a try if performance is not compromised. Currently use XFS.
Again not speaking to the project itself, but in principle achieving good performance on something like this would boil down to “do what SQL databases do, then design efficient schemas and queries for the use case”.
Fortunately you can try Supertag out without touching your original files, as Supertag will use symlinks to your original files, so you don't need to move them.