They could. But if they filed a claim under the CFAA without ever sending a cease and desist letter to the alleged intruder, I think the claim would be dismissed.
Is simply changing TOS enough for a CFAA claim to have a reasonable chance of success. I could be wrong, but I believe for every CFAA claim we have seen so far based on "scraping", there was some notice to stop directed specifically at the respondent. If someone thinks just changing TOS (public notice) is enough for a CFAA claim to survive a Motion to Dismiss and there is no need to also contact the alleged offender asking them to stop, then let's hear about the precedent that supports that idea. I do not think there is any such precedent, but I could be wrong.