The reasons this doesn't work for datacenters is two-fold, I think: First, they won't see efficiency improvements just by keeping their CPUs and GPUs (or RAM) cooler because the power levels/tables for the chips are baked-in, and operators aren't going to the trouble of tweaking voltages themselves. Second, even if they did tweak voltages, the cost of sustaining lower temperatures with better cooling likely won't outweigh the savings resulting from lower power draw for the chips.
Still, this raises the question of whether designing hardware for higher operating temperatures is always the right move. At some point there's going to be a cost in performance and/or efficiency that outweighs the savings from allowing higher temperatures. Ideally these tradeoffs should be balanced as a whole.