High frequency radars are more accurate than low frequency, nobody used low frequency at the time. They're also smaller, I don't think you could use a low frequency radar with a missile's seeker. Low frequency is good enough to throw up flak, though--and that's how the one that was lost got hit.
It was also vulnerable to bistatic radar--but I don't believe a bistatic radar could even have been built back then.
It was basically a one-trick wonder that got counterdesigned.