I’ve heard really good things about SuperH (sh-2, sh-4 etc.), designed by Hitachi for their processors including those used in the Sega Saturn and Sega Dreamcast. Really high code density was one big thing, but it was covered by patents until recently. There was a group trying to make a modern open source processor in VHDL for FPGAs and later on ASICs based on it, but I think it may have mostly fizzled out.