If you watch this video[0], you'll see in the first frame that there is a clear boundary between learning rates that converge or not. Ignoring this paper for a moment, what if we zoom in really really close to that boundary? There are two possibilities, either (1) the boundary is perfectly sharp no matter how closely we inspect it, or (2) it is a little bit fuzzy. Of those two possibilities, the perfectly sharp boundary would be more surprising.
And indeed, the AI response indicated that the boundary between convergence and divergence is not well defined, has many local maxima and minima, and could be quote: "fractal or chaotic, with small changes in hyperparameters leading to drastically different outcomes."