I've always loved What Dreams May Come and felt similarly about The Fountain. Do you have any other recommendations?
Try 2006's The Fall for another special film that surprises your heart and gives a visual treat.
People are probably already aware of the fact, but it is based on a novel of the same name by Richard Matheson — who also wrote I Am Legend (which has had its own fair share of film adaptations).
I liked the visuals in Life of Pi a lot. Also, The Secret Life of Walter Mitty, for obvious reasons.