You don't have to try hard. Just use it as a photodiode and it magically works. However, if it's inside a plastic case that blocks light, it doesn't.

Due to some law about entropy, efficient processes are necessarily reversible. That's why electric motors - some of the most efficient machines ever invented - are also generators.

Especially true for LEDs, tried that in the lab once with a flood light, got a few μA out of the LED shortened with the multimeter. Did that with 8th graders, we did other experiments mainly with pv, LEDs and bipolar transistors as well.

The logical question came up more than once: “can we use photovoltaic cells as a light?“. Pretty sure that‘ll work, too, but didn’t try because stuff was expensive then and we didn’t have any broken parts of cells at the time. They probably learned a few things on that day.