That said, your comment stands out to me to be self-contradictory and unscientific (by way of being alarmist and not backing up an extraordinary claim ).
> Unknown second order effects
This sounds right.
> Nearest real world success is continuous low volume maritime dispersal which has completely different dispersal dynamics than high-altitude bursts, and the continuous low volume maritime dispersal is non-viable
Since I don't know a lot about this topic I'll take your word for it.
> No way to undo it once done
This doesn't sound quite right, my intuition says more likely "no known way to undo it once done".
> If humans can’t perpetually release aerosols — and I mean perpetually, for the next millions of years — then the global climate “snaps back” violently within weeks
Wait... So, to undo it all we have to do is stop doing it? Doesn't this contradict the statement right before it?
> almost certainly eradicates all known life in the entire universe
This statement makes me suspicious of the credibility of the rest. This is an extraordinary claim and I think deserves way more explanation if you want to convince anyone who doesn't already agree with you. It would be a lot easier to accept "decimates human civilization" than "eradicate all life on earth". Life is extremely resilient.
How exactly would it eradicate all life on earth?