Literate programming is not about programming in natural languages: it's about integrating code (i.e. the formal description in some DSL) with the meta-code such as comments, background information, specs, tests, etc.

BTW, one side benefit of LP is freedom from arbitrary structure of DSLs. A standard practice in LP is to declare and define objects in the spot in which they are being used; LP tools will parse them out and distribute to the syntactically correct places.