the very point of brutalism is to turn its material 'inside out', what defines brutalism is that it makes the material and structural elements it's made of visible. It's not a 'visual style' or an aesthetic at all but an 'ethic of construction' something was brutalist if it was honest, and exposed, what a thing was made of.
If you want to apply that notion to web design It's not about 1 CSS file or 100 but whether the mechanics of CSS or HTML are still visible on the site, or if it's all buried under colors, animations, styling etc. Craigslist is a pretty good example of a brutalist website, so is this site, HN.