Datasets like those can be used for fine tuning a pretrained LLM towards a specific domain, but for decent (not even state of art, just anything usable) results you need a large enough dataset to learn English and general world knowledge, and for that the preferable size is "almost everything you can get your hands on", as in, the quantity you'd want to train on is larger than the quantity of good data you can realistically get. Like, the 800 GiB of text at https://pile.eleuther.ai/ is a good start, but if you could get ten times more data (as some of the big companies probably do, since they have access to lots of user-generated non-public text), you should definitely use that.
If you want targeted LLMs then IMHO the proper mindset for data choice is "take everything that you can out of what humanity has ever written and then pick out of that the most suitable 20% for your needs" and that would give much better results than any single dataset that's only Wikipedia-sized.