The longer the half life, the lower the power output, no free lunches. But by putting the same suitable radioactive lump in a stirling engine you can extract 4 times as much electricity: https://en.wikipedia.org/wiki/Stirling_radioisotope_generato...
So yes maybe with Americium-241 we could have something which lasts 4 times a much _and_ gives us the same amount of power thanks to a SRG.