RIP. My favourite Spassky game is this 24 move win against Petrosian and Petrosian was no patzer: https://www.chessgames.com/perl/chessgame?gid=1106864
Also it was probably not objectively the best move (and definitely not Spassky's best game) but Tim Krabbé made a list of 110 most fantastic moves ever played, and he put Spassky's 16...Nc6 against Averbakh as no. 1 (certainly an unorthodox choice):